生态与农村环境学报 ›› 2014, Vol. 30 ›› Issue (6): 699-705.doi:

• 区域环境与发展 • 上一篇    下一篇

珠江流域湖库型水源集水区酞酸酯(PAEs)类污染物环境健康风险评估

贺涛,许振成,魏东洋,白中炎,任明忠,白小舰   

  1. 环境保护部华南环境科学研究所
  • 收稿日期:2014-01-17 修回日期:2014-10-13 出版日期:2014-11-25 发布日期:2014-12-05
  • 通讯作者: 魏东洋 环境保护部华南环境科学研究所 E-mail:weidongyang@scies.org
  • 作者简介:贺涛(1981—),男,江西永新人,高级工程师,博士,主要从事饮用水源环境评估与风险管理研究。E-mail:hetao@scies.org
  • 基金资助:

    国家环保公益性行业科研专项(201109015,2013467042)

Environmental Health Risk Assessment of Phthalic Acid Esters Like Pollutants in Reservoir or Lake Type Water Source Catchments in the Pearl River Basin

HE  Tao, XU  Zhen-Cheng, WEI  Dong-Yang, BAI  Zhong-Yan, REN  Ming-Zhong, BAI  Xiao-Jian   

  1. South China Institute of Environmental Sciences,Ministry of Environmental Protection
  • Received:2014-01-17 Revised:2014-10-13 Online:2014-11-25 Published:2014-12-05
  • Contact: WEI Dong-Yang South China Institute of Environmental Sciences,Ministry of Environmental Protection E-mail:weidongyang@scies.org

摘要:

以饮用水源集水区为中心,沿支流采集水样,采用美国环境保护署(USEPA)暴露风险评价方法,结合该地区的参数计算环境健康风险。结果表明:(1)所有采样点均检出PAEs 类污染物邻苯二甲酸正丁酯(DBP)、邻苯二甲酸二(2-乙基己基)酯(DOP)和邻苯二甲酸二酯(DEP),其中DOP 高于DBP 和DEP。(2)该饮用水源集水区3 种PAEs 污染物质量浓度均高于流域内其他乡镇饮用水源,在国内外同类地区也属于中上水平。DOP 是集水区内需首要控制的PAEs 类污染物。(3)在人类活动干扰少的地区河流污染物的环境健康风险水平较低,而在人口密集区和工业集中区风险水平较高。河流上游风险值低,中游高,下游和库区又逐渐回落。该水源集水区的PAEs类污染物环境健康风险值未超过USEPA 规定,但与国内外其它地区相比属于中上水平,存在一定的潜在健康风险,需要根据PAEs 的可能来源在水源地环境风险管理中加以防范。

关键词: PAEs, 水源集水区, 健康风险评估

Abstract:

Water samples were collected along the tributaries of a drinking water source catchment for analysis in line with the procedure for risk assessment of the USEPA, and environment health risk of phthalic acid esters (PAEs) was assessed by taking into account the parameters of the region. Results show that (1) all the samples were found to have PAEs like pollutants, including Di (2-ethylhexyl) phthalate (DOP), diethyl phthalate (DEP), di-n-butyl phtalate (DBP), among which DOP was higher than the other two, displaying an order of DOP > DEP > DBP.  (2) The concentrations of DOP, DEP and DBP in the water catchment were all higher than their respective ones in other drinking water source catchments in the region and could also be sorted into the moderate or upper level of contamination in similar areas in the country and others. DOP was designated the primarily controlled contaminant of the water source catchment.(3) In areas less affected by anthrogenic disturbance, environmental health risk of pollutants in rivers was low, while in areas densely populated and concentrated with industry, the risk was high. Along a river, the risk was low in the upper reaches, high in the middle reaches and low again in the lower reaches or the reservoirs.Therefore, it can be concluded that the environment health risk of PAEs like contaminants in headwater catchment has not yet exceeded the criteria of USEPA, but among similar regions the world over, this region is moderate or high in concentration of PAEs like contaminants and does have some potential health risks. It is, therefore, essential to track potential source of PAEs in the region and take corresponding countermeasures to control the sources in environmental risk management of the region.

Key words: PAEs(phthalic acid esters), water source catchment, environmental health risk assessment

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