生态与农村环境学报 ›› 2023, Vol. 39 ›› Issue (9): 1133-1143.doi: 10.19741/j.issn.1673-4831.2022.0875

• 区域环境与发展 • 上一篇    下一篇

基于Kolmogorov-Zurbenko滤波法分析2015—2021年京津冀地区大气颗粒物变化趋势

占青, 张运江, 陈红, 张可馨, 盖鑫磊   

  1. 南京信息工程大学环境科学与工程学院/江苏省大气环境监测与污染控制高技术研究重点实验室/大气环境与装备技术协同创新中心, 江苏 南京 210044
  • 收稿日期:2022-08-24 出版日期:2023-09-25 发布日期:2023-09-19
  • 通讯作者: 张运江,E-mail:yjzhang@nuist.edu.cn E-mail:yjzhang@nuist.edu.cn
  • 作者简介:占青(1999-),女,江苏盐城人,主要研究方向为大气环境。E-mail:15251031203@163.com
  • 基金资助:
    江苏省自然科学基金(BK20210663);国家环境保护城市大气复合污染成因与防治重点实验室开放基金(CX2020080579)

Trend Analysis of Atmospheric Particulate Matter over the Beijing-Tianjin-Hebei Region During 2015-2021 Using the KZ Filtering Approach

ZHAN Qing, ZHANG Yun-jiang, CHEN Hong, ZHANG Ke-xin, GE Xin-lei   

  1. School of Environmental Science and Engineering, Nanjing University of Information Science and Technology/Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control/Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Nanjing 210044, China
  • Received:2022-08-24 Online:2023-09-25 Published:2023-09-19

摘要: 京津冀地区是我国近年针对大气颗粒物污染治理的重点区域。采用Kolmogorov-Zurbenko(KZ)滤波分析2015-2021年京津冀地区13个城市细颗粒物(PM2.5)、可吸入颗粒物(PM10)和粗颗粒物(PM2.5-10)的时间序列。结果表明,PM2.5和PM10年均浓度总体呈下降趋势,其下降速率分别为5.07和8.10 μg·m-3·a-1。KZ滤波分析结果表明,PM2.5、PM10和PM2.5-10的短期分量、季节分量和长期分量之间相互独立。短期分量贡献占比(大于50%)最高,其次为季节分量,说明原始时间序列的波动主要受控于污染源排放以及气象条件的短期变化和季节变化。针对KZ滤波分解出的浓度序列,建立逐步多元回归线性模型,定量评估气象和减排对变化趋势的贡献。逐城分析结果表明,秦皇岛市气象条件对PM2.5浓度的影响(14.86%)最大,衡水市减排措施对PM2.5浓度的影响(96.77%)最大;秦皇岛市气象条件对PM10浓度的影响(13.69%)最大,廊坊市减排措施对PM10浓度的影响(93.96%)最大;沧州市气象条件对PM2.5-10浓度的影响(26.23%)最大,廊坊市减排措施对PM2.5-10浓度的影响(91.80%)最大。整体分析结果表明,减排对2015-2021年京津冀大气颗粒物污染改善起着至关重要的作用。

关键词: 大气颗粒物, KZ滤波法, 逐步多元线性回归, 变化趋势, 京津冀地区

Abstract: The Beijing-Tianjin-Hebei Region has become a key focus area for addressing atmospheric particulate matter pollution in recent years in China. In this study, Kolmogorov-Zurbenko (KZ) filtering analysis was applied to analyze the time series of fine particulate matter (PM2.5), inhalable particulate matter (PM10), and coarse particulate matter (PM2.5-10) in 13 cities in the Beijing-Tianjin-Hebei Region from 2015 to 2021. The results show that the annual average concentrations of PM2.5 and PM10 had generally decreased, with a decline rate of 5.07 and 8.10 μg·m-3·a-1, respectively. The KZ filtering analysis also revealed that the short-term, seasonal, and long-term components of PM2.5, PM10, and PM2.5-10 are independent of each other. The highest contribution to the fluctuations in the original time series was found to be from the short-term component (over 50%), followed by the seasonal component, indicating that the fluctuations are mainly influenced by short-term and seasonal variations in pollutant emissions and meteorological conditions. Using the KZ-filtered concentration series, a stepwise multiple regression linear model was established to quantitatively evaluate the contributions of meteorological factors and emission reduction measures to the trends observed. The city-by-city analysis results show that the impact of meteorological conditions on PM2.5 concentrations was highest in Qinhuangdao (14.86%), while emission reduction measures had the greatest impact on PM2.5 concentrations in Hengshui (96.77%). The impact of meteorological conditions on PM10 concentrations was highest in Qinhuangdao (13.69%), while emission reduction measures had the greatest impact on PM10 concentrations in Langfang (93.96%). The impact of meteorological conditions on PM2.5-10 concentrations was highest in Cangzhou (26.23%), while emission reduction measures had the greatest impact on PM2.5-10 concentrations in Langfang (91.80%). Overall, the analysis results suggest that emission reduction measures plays a crucial role in improving particulate matter pollution in the Beijing-Tianjin-Hebei Region from 2015 to 2021.

Key words: atmospheric particulate matter, KZ filtering, stepwise multiple linear regression, trend change, Beijing-Tianjin-Hebei Region

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